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There was no instance at any point throughout the series when Aang, Katara, Toph and Sokka had a battle against the Dai Li. Aang and Katara battled the entire army under Ba Sing Se's catacombs in "The Crossroads of Destiny", but were unable to defeat them. Later on, Aang, Toph and Sokka battled two of Azula's Dai Li agents in the "The Day of Black Sun, Part 2: The Eclipse", where Toph was able to defeat both easily.

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